Special Issue on Carbonaceous Aerosols in the Atmosphere (II)

Sultan F.I. Abdillah1,2,3, Sheng-Jie You2,3, Ya-Fen Wang This email address is being protected from spambots. You need JavaScript enabled to view it.2,4 

1 Department of Civil Engineering, Chung Yuan Christian University, Zhongli, Taoyuan 32023, Taiwan
2 Department of Environmental Engineering, Chung Yuan Christian University, Zhongli, Taoyuan 32023, Taiwan
3 Center for Environmental Risk Management, Chung Yuan Christian University, Zhongli, Taoyuan 32023, Taiwan
4 Sustainable Environmental Education Center, Chung Yuan Christian University, Zhongli, Taoyuan 32023, Taiwan


 

Received: November 29, 2023
Revised: January 28, 2024
Accepted: February 28, 2024

 Copyright The Author(s). This is an open access article distributed under the terms of the Creative Commons Attribution License (CC BY 4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are cited.


Download Citation: ||https://doi.org/10.4209/aaqr.230295  


Cite this article:

Abdillah, S.F.I., You, S.J., Wang, Y.F. (2024). Characterizing Traffic-Related Ultrafine Particles in Roadside Microenvironments: Spatiotemporal Insights from Industrial Parks. Aerosol Air Qual. Res. 24, 230295. https://doi.org/10.4209/aaqr.230295


HIGHLIGHTS

  • Seasonal measurement campaigns were conducted at roadsides and urban background.
  • Roadsides possess different semi-diurnal profile compared to urban background.
  • Elevated particles concentrations were found during cold seasons & peak periods.
  • Roadsides ultrafine particles might possess intra-urban spatial variability.
  • Traffic profiles and meteorological data significantly influence particles concentrations.
 

ABSTRACT


Ultrafine particles (UFPs; PM0.1) and black carbon (BC) were measured at different roadside microenvironments in the vicinity of the urban industrial park area. Simultaneous measurement campaigns were conducted at industrial roadside (IN), residential roadside (RS), and urban background (UB) throughout different seasons. Spatiotemporal variability as well as correlations between pollutants and confounding factors (traffic profiles and meteorological conditions) were analyzed. The observed average roadside UFPs particle number concentration (UFPs PNC) and BC concentrations were in the order of IN (38,000 ± 9,000 # cm–3 and 2,500 ± 600 ng m–3) > RS (25,000 ± 8,000 # cm–3 and 1,900 ± 300 ng m–3) > UB (23,000 ± 9,000 # cm–3 and 1,400 ± 300 ng m3). Furthermore, 11.26%–16.06% and 20.35%–24.32% increases of the average UFPs PNC and BC mass concentrations were identified during cold period at all measurement sites. Additionally, peak average concentrations of UFPs PNC and BC were identified at IN and RS during morning rush-hour and weekdays periods, following the diurnal profiles of traffic flux compositions and total vehicle number per day. Intra-urban spatial variability of UFPs was identified between roadsides and urban background (IQR/M ratio ≥ 2, ρ ≤ 0.05), highlighting the heterogeneity characteristic of the pollutant. Both pollutants at IN and RS were significantly influenced by traffic activities, while at UB, they were associated with meteorological conditions and secondary emission. Elevated levels of pollutants identified in this study have exceeded typical “high-level” UFPs according to WHO AQG 2021, indicating an intensified exposure risk for pedestrians and residents. This study serves as reference for future epidemiological study related to roadside UFPs in typical urban microenvironments such as industrial park areas.


Keywords: Black carbon, Roadside microenvironments, Spatiotemporal variability, Ultrafine particles, Urban industrial park




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