Suyi Hou1, Weihan Li1, Liudongqing Yang2, Guorong Chen1,2, Yilin Zhang2, Mikinori Kuwata  This email address is being protected from spambots. You need JavaScript enabled to view it.1,2

1 Department of Atmospheric and Oceanic Sciences and Laboratory for Climate and Ocean-Atmosphere Studies, School of Physics, Peking University, Beijing 100871, China
2 Earth Observatory of Singapore and the Asian School of Environment, Nanyang Technological University, Singapore 639798, Singapore


Received: July 3, 2022
Revised: September 6, 2022
Accepted: December 19, 2022

 Copyright The Author(s). This is an open access article distributed under the terms of the Creative Commons Attribution License (CC BY 4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are cited.


Download Citation: ||https://doi.org/10.4209/aaqr.220265  


Cite this article:

Hou, S., Li, W., Yang, L., Chen, G., Zhang, Y., Kuwata, M. (2023). The Role of Sulfur Emission from the Petroleum Industry on Ultrafine Particle Number Concentration in Singapore. Aerosol Air Qual. Res. 23, 220265. https://doi.org/10.4209/aaqr.220265


HIGHLIGHTS

  • A year-long observation of ultrafine particle was conducted in Singapore.
  • Both primary and secondary sources of ultrafine particles were identified.
  • Ultrafine particle number concentration increased for SO2-rich air masses.
 

ABSTRACT


Ultrafine particles, defined as particles with a diameter (dp) smaller than 100 nm, serve as an important component of cloud condensation nuclei, in addition to impacting human health. The dominant sources of ultrafine particles include traffic emissions and nucleation. Singapore is a tropical city that hosts petrochemical industries. To identify the sources of ultrafine particles, a year-long observation of the number size distribution was conducted in Singapore in 2018 and 2019. The concentrations of CO, CO2, CH4, and SO2 were also monitored. The particle number concentration during the southwest monsoon season was high, while that during the northeast monsoon period was relatively low. The CO concentration increased during the morning traffic rush hours, which was associated with relatively minor enhancements in ultrafine particle number concentration. The events for a high number concentration of the Aitken mode particles (dp < 50 nm) were identified during high SO2 concentration periods. The SO2 concentration was high during the afternoon because the sea breeze transported the emissions from the coastal industrial area to the observation site. The enhancements in CH4 from its background level (ΔCH4) and SO2 had a quasi-inverse relationship, as the major emission sources of these two chemical species were different. The particle number concentration (dp > 50 nm) correlated with the enhancements in CO concentration (ΔCO) for CH4-dominant air masses, suggesting that incomplete combustion processes, such as traffic emission, are important for the size range. Conversely, the number concentration of the Aitken mode particles (dp < 50 nm) increased for SO2-dominant air masses, suggesting the importance of industrial plume.


Keywords: Singapore, Ultrafine particles, New particle formation, Sulfur dioxide




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