Eun Hee Jo1,2, Sun Kyung Kim1, Hankwon Chang1,2, Chongmin Lee1, Su-Ryeon Park1, Ji-Hyuk Choi2, Hee Dong Jang This email address is being protected from spambots. You need JavaScript enabled to view it.1,2


Resources Utilization Research Center, Korea Institute of Geoscience and Mineral Resources, Yuseong-gu, Daejeon 34132, Korea
Department of Nanomaterials Science and Engineering, University of Science and Technology, Yuseong-gu, Daejeon 34113, Korea


Received: October 17, 2018
Revised: October 17, 2018
Accepted: November 19, 2018

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Jo, E.H., Kim, S.K., Chang, H., Lee, C., Park, S.R., Choi, J.H. and Jang, H.D. (2019). Synthesis of Multiwall Carbon Nanotube/Graphene Composite by an Aerosol Process and its Characterization for Supercapacitors. Aerosol Air Qual. Res. 19: 449-454.


  • MWNT/GR composite was fabricated by aerosol spray drying.
  • The composites showed a crumpled paper ball like morphology.
  • The composite electrode showed excellent capacitance and rate of capacity retention.


A multiwall carbon nanotube/graphene (MWCNT/GR) composite was synthesized for an enhanced supercapacitor. Aerosol spray drying (ASD) was used to synthesize the MWCNT/GR particles using a mixture of graphene oxide (GO) solution and MWCNT. The effect of the MWCNT/GO ratio on the properties of the composite, including its shape and structure, was investigated. The composite particles were generally shaped like a crumpled paper ball, with an average diameter of approximately 5 µm. The MWCNTs, which were uniformly dispersed among the graphene sheets, not only increased the basal spacing of the sheets but also bridged the wide gaps between them, thereby improving electron transfer between the layers. Thus, the MWCNTs increased the contact area of the electrolyte/electrode and facilitated the transportation of electrons and electrolyte in the electrode. Using a two-electrode testing system, the electrochemical results demonstrate that the MWCNT/GR (weight ratio = 0.1) electrode has a capacitance of 192 F g–1 and an excellent rate of capacity retention (88% at 4 A g–1).

Keywords: Supercapacitor; MWCNT/GR; Aerosol spray drying.

Aerosol Air Qual. Res. 19 :449 -454 .  

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