Oliver V. Rattigan 1, Kevin L. Civerolo1, H. Dirk Felton1, James J. Schwab2, Kenneth L. Demerjian2

  • 1 New York State Department of Environmental Conservation, Division of Air Resources, (null), USA
  • 2 Atmospheric Sciences Research Center, University at Albany, State University of New York, (null), USA

Received: May 14, 2015
Revised: September 30, 2015
Accepted: October 12, 2015
Download Citation: ||https://doi.org/10.4209/aaqr.2015.05.0319  


Cite this article:
Rattigan, O.V., Civerolo, K.L., Felton, H.D., Schwab, J.J. and Demerjian, K.L. (2016). Long Term Trends in New York: PM2.5 Mass and Particle Components. Aerosol Air Qual. Res. 16: 1191-1205. https://doi.org/10.4209/aaqr.2015.05.0319


HIGHLIGHTS

  • Trends in PM2.5 mass and major particle components over a 14–15 yr period.
  • Annual urban PM2.5 mass decreased by 30–40% and rural by 25–30%.
  • Particle SO4 and NO3 accounted for most of the PM2.5 reductions.
  • Air quality improvements attributed to emission controls on SO2 and NOx.
  • OC showed little change and is currently the major component of PM2.5 mass.

 

ABSTRACT


Measurements of PM2.5 mass and particle components over a 14–15 year period are used to explore trends at urban and rural locations across New York State. Such data are used to determine compliance with national ambient air quality standards (NAAQS), as well as track the effectiveness of reductions in source pollutant emissions. Since 2000 annual mean PM2.5 mass shows a downward trend with decreases of 4–7 µg m–3 in urban areas versus 3–4 µg m–3 for rural background sites. Much of this change can be attributed to particle sulfate (SO4) and nitrate (NO3) which showed annual decreases of 2–3 µg m–3 and 0.5–1.0 µg m–3, respectively. Determining accurate trends for the carbonaceous particle material is challenging due to the changes in the carbon sampling and analysis methods which impact the measurements. Analysis of the data indicate some decreases in particle elemental carbon (EC) but little change in the organic carbon fraction (OC). Significant improvements in air quality are observed since 2000, when New York City metropolitan area exceeded the 1997 annual PM2.5 standard of 15 µg m–3, to the present conditions where it meets the current standard of 12 µg m–3. Further improvements in air quality may benefit from controls on carbonaceous material which is currently the major component of PM2.5.


Keywords: PM2.5 mass; Long term trends; Particle species; Major ions; Air monitoring


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