OPEN ACCESS

Articles online

Characteristic and Compositions of Airborne Fine Particulate Matter in the Southwest Ohio, USA

Category: Urban Air Quality

Accepted Manuscripts
DOI: 10.4209/aaqr.2017.08.0256
PDF | RIS | BibTeX

Chunjuan Xie1,2, Mingming Lu 2, Kaiqi Li2, Jian Li2,3, Anna L. Kelley4

  • 1 College of Science, East China Jiaotong University, Nanchang 330013, China
  • 2 Department. of Chemical and Environmental Engineering, University of Cincinnati, Cincinnati, OH 45221, USA
  • 3 Key Laboratory of Jiangxi Province for Persistant Pollutants Control and Resources Recycle, School of Environmental and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, China
  • 4 Monitoring and Analysis Supervisor, Southwest Ohio Air Quality Agency, Cincinnati, OH 45219, USA

Highlights

The total concentration of PM2.5 decreased significantly since the last decade.
The most dominant components of PM2.5 were sulfates, OM, and nitrates.
The highest sulfate concentrations occur in the summer.
The highest nitrates occur in the winter.
Sulfate in Cincinnati is in high level, still needs to make great effort to control.


Abstract

The Southwest Ohio has been known for PM2.5 issues due to emissions from multiple local sources, such as industry and multimodal traffic, as well as regional impacts from sulfates, nitrates and ammonia. To better understand the speciation characteristics of PM2.5 in Southwest Ohio area, data from five monitoring sites, Taft, Hook Field, St. Bernard, Lower Price Hill, and Chase were studied for the time period of 2003 to 2013. The total concentration of PM2.5 has decreased significantly since the last decade, from 13.41 µg m–3 in 2003 to 10.55 µg m–3 in 2013. The overall PM2.5 concentration also exhibited seasonal variations, with four out of five of the highest concentrations occurring in summer, and the fifth one in winter. With various air pollution control measures (such as Cross State Air Pollution Rule Mercury and Air Toxics Standards), both the total concentrations and the speciation of PM2.5 have changed overtime. The most dominant components of PM2.5 include sulfates, organic matter (OM), and nitrates, which are 33.4%, 31.7% and 17.7% respectively (Taft data from 2009 to 2013). Elemental carbon (EC) and crustal materials, on the other hand, took much smaller portions of 2.84% and 3.61%, respectively. The highest sulfate concentrations occured in the summer, while those for nitrates occured in the winter. EC and OM followed the same seasonal trends, which peaked in the fall and summer, and were the lowest in winter. Crustal materials exhibited the lowest concentrations in winter. Comparison of the Cincinnati, (Taft site) with other major cities nearby indicated that PM2.5 in Cincinnati is higher and the fraction of sulfates is the largest. Efforts to control its emission are still necessary.

Keywords

PM2.5 Chemical speciation Southwest Ohio Sulfate


Related Article

Seasonal Source Apportionment of PM2.5 in Ningbo, a Coastal City in Southeast China

Mengren Li, Min Hu , Qingfeng Guo, Tianyi Tan, Bohan Du, Xiaofeng Huang, Lingyan He, Song Guo, Weifeng Wang, Yingguo Fan, Dandan Xu
Accepted Manuscripts
DOI: 10.4209/aaqr.2018.01.0011
PDF

Spatio-temporal Variations in NO2 and PM2.5 over the Central Plains Economic Region of China during 2005-2015 Based on Satellite Observations

Kun Cai, Shenshen Li , Fengbin Zheng , Chao Yu, Xueying Zhang, Yang Liu, Yujing Li
Volume: 18 | Issue: 5 | Pages: 1221-1235
DOI: 10.4209/aaqr.2017.10.0394
PDF

Observation Analysis on Microphysics Characteristics of Long-lasting Severe Fog and Haze Episode at Urban Canopy Top

Su-Qin Han , Tian-Yi Hao, Min Zhang, Qing Yao, Jing-Le Liu, Zi-Ying Cai, Xiang-Jin Li
Accepted Manuscripts
DOI: 10.4209/aaqr.2017.10.0416
PDF

Meteorological Overview and Signatures of Long-range Transport Processes during the MAPS-Seoul 2015 Campaign

Cheol-Hee Kim , Hyo-Jung Lee, Jeong-Eon Kang, Hyun-Young Jo, Shin-Young Park, Yu-Jin Jo, Jong-Jae Lee, Geum-Hee Yang, Taehyun Park, Tae-Hyung Lee
Accepted Manuscripts
DOI: 10.4209/aaqr.2017.10.0398
PDF
;